One vertex per element, one color per generator, with an edge from x to x·s.
(1,2)(3,15)(4,21)(5,27,30,41)(6,13)(7,12)(8,14)(9,18)(10,24)(11,29,42,31)(16,36)(17,48,50,40)(19,34)(20,35)(22,32)(23,37,55,63)(25,39)(26,38)(28,44,51,33)(43,47)(45,61,49,59)(46,60)(52,54,57,56)(53,62,58,64)(1,3)(2,9,14,15)(4,22)(5,28,30,51)(6,20)(7,19)(8,18)(10,36,39,60)(11,40)(12,35,13,34)(16,25)(17,29,50,31)(21,43,38,32)(23,49,55,45)(24,46)(26,47)(27,33)(37,61)(41,44)(42,48)(52,64)(53,54,58,56)(57,62)(59,63)(1,4,6,24,8,26,7,25)(2,10,12,21,14,39,13,38)(3,16,19,47,18,46,20,22)(5,23,29,54,30,55,31,56)(9,32,34,60,15,43,35,36)(11,37,41,52,42,63,27,57)(17,49,51,53,50,45,28,58)(33,61,48,62,44,59,40,64)(1,5)(2,11)(3,17,18,50)(4,23)(6,29)(7,31)(8,30)(9,33,15,44)(10,37)(12,41)(13,27)(14,42)(16,45,46,49)(19,51,20,28)(21,52)(22,53,47,58)(24,54)(25,56)(26,55)(32,59,43,61)(34,48,35,40)(36,62,60,64)(38,57)(39,63)A Cayley diagram is a choice, not a fact about the group. Another drawing of this group — in a book, or on a different generating set — may look nothing like this one.