One vertex per element, one color per generator, with an edge from x to x·s.
(1,2)(3,13,17,42)(4,9,20,35)(5,21)(6,11)(7,12)(8,16,31,44)(10,25)(14,43)(15,48,50,36)(18,33,54,61)(19,34,26,39)(22,57,52,30)(23,37,55,56)(24,40)(27,38)(28,32)(29,51)(41,47)(45,63)(46,59)(49,58)(53,62)(60,64)(1,3)(2,8,12,31)(4,14,20,47)(5,22)(6,16)(7,17)(9,29)(10,36,21,48)(11,13,32,42)(15,27)(18,53,54,49)(19,46,26,51)(23,45,55,64)(24,50)(25,52)(28,44)(30,40,57,38)(33,60)(34,43)(35,59)(37,62)(39,41)(56,58)(61,63)(1,4,6,26,7,20,28,19)(2,9,32,34,12,35,11,39)(3,14,44,46,17,47,16,51)(5,23,27,54,25,55,24,18)(8,29,13,41,31,59,42,43)(10,37,38,33,21,56,40,61)(15,49,22,45,50,53,52,64)(30,60,36,62,57,63,48,58)(1,5,6,27,7,25,28,24)(2,10,32,38,12,21,11,40)(3,15,44,22,17,50,16,52)(4,18,26,23,20,54,19,55)(8,30,13,36,31,57,42,48)(9,33,34,56,35,61,39,37)(14,45,46,53,47,64,51,49)(29,58,41,60,59,62,43,63)A Cayley diagram is a choice, not a fact about the group. Another drawing of this group — in a book, or on a different generating set — may look nothing like this one.