One vertex per element, one color per generator, with an edge from x to x·s.
(1,2,9,15)(3,16,20,37)(4,21)(5,28,30,45)(6,31,7,13)(8,12,29,14)(10,32,39,19)(11,24)(17,35)(18,46,55,36)(22,57)(23,47)(25,44)(26,41)(27,43)(33,49,60,38)(34,42)(40,59)(48,53)(50,64)(51,56)(52,61)(54,62)(58,63)(1,3,6,19,9,20,7,32)(2,10,13,16,15,39,31,37)(4,22,24,51,27,59,25,58)(5,18,8,33,30,55,29,60)(11,40,21,56,44,57,43,63)(12,36,28,49,14,46,45,38)(17,50,52,23,54,34,53,26)(35,47,48,64,62,41,61,42)(1,4)(2,11,15,44)(3,17,20,54)(5,23)(6,24)(7,25)(8,34)(9,27)(10,35)(12,41,14,47)(13,21,31,43)(16,48)(18,51,55,58)(19,52,32,53)(22,33,59,60)(26,30)(28,42,45,64)(29,50)(36,40)(37,61)(38,63)(39,62)(46,57)(49,56)(1,5,7,29,9,30,6,8)(2,12,31,45,15,14,13,28)(3,18,32,60,20,55,19,33)(4,23,25,50,27,26,24,34)(10,36,37,38,39,46,16,49)(11,41,43,64,44,47,21,42)(17,51,53,22,54,58,52,59)(35,40,61,63,62,57,48,56)A Cayley diagram is a choice, not a fact about the group. Another drawing of this group — in a book, or on a different generating set — may look nothing like this one.